Rare earth oxides and their supported noble metals in application of environmental catalysis
来源期刊：JOURNAL OF RARE EARTHS2020年第8期
论文作者：Zhiquan Hou Wenbo Pei Xing Zhang Kunfeng Zhang Yuxi Liu Jiguang Deng Lin Jing Hongxing Dai
文章页码：819 - 839
摘 要：Volatile organic compounds（VOCs）,methane,carbon monoxide,soot,automotive exhaust,and nitrogen oxides are harmful to the atmosphere and human health.It is urgent to strictly control their emissions.Heterogeneous catalysis is an effective pathway for the removal of these pollutants,and the critical issue is the development of novel and high-performance catalysts.In this review,we briefly summarize the preparation methods,physicochemical properties,catalytic activities,and related reaction mechanisms for the above pollutants removal of the rare earth oxides,mixed rare earth oxide,rare earth oxidesupported noble metal,and mixed rare earth oxide-supported noble metal catalysts that have been investigated by our group and other researchers.It was found that catalytic performance was associated with the factors,such as specific surface area,pore structure,particle size and dispersion,adsorbed oxygen species concentration,reducibility,reactant activation ability or interaction between metal nanoparticles and support.Furthermore,we also envision the development trend of such a topic in future work.
Zhiquan Hou，Wenbo Pei，Xing Zhang，Kunfeng Zhang，Yuxi Liu，Jiguang Deng，Lin Jing，Hongxing Dai
Beijing Key Laboratory for Green Catalysis and Separation,Key Laboratory of Beijing on Regional Air Pollution Control,Key Laboratory of Advanced Functional Materials,Education Ministry of China,Laboratory of Catalysis Chemistry and Nanoscience,Department of Chemistry and Chemical Engineering,College of Environmental and Energy Engineering,Beijing University of Technology
摘 要：Volatile organic compounds（VOCs）,methane,carbon monoxide,soot,automotive exhaust,and nitrogen oxides are harmful to the atmosphere and human health.It is urgent to strictly control their emissions.Heterogeneous catalysis is an effective pathway for the removal of these pollutants,and the critical issue is the development of novel and high-performance catalysts.In this review,we briefly summarize the preparation methods,physicochemical properties,catalytic activities,and related reaction mechanisms for the above pollutants removal of the rare earth oxides,mixed rare earth oxide,rare earth oxidesupported noble metal,and mixed rare earth oxide-supported noble metal catalysts that have been investigated by our group and other researchers.It was found that catalytic performance was associated with the factors,such as specific surface area,pore structure,particle size and dispersion,adsorbed oxygen species concentration,reducibility,reactant activation ability or interaction between metal nanoparticles and support.Furthermore,we also envision the development trend of such a topic in future work.
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